Library of Congress is listed below that. Open EndNote 20, on the left pane, there is a category called ONLINE SEARCH.To search the LC catalog from EndNote, here are the steps: If what you want to search for is a book reference, you may search for it in the Library of Congress (LC) online catalog. Users are recommended to use EndNote 20 for this feature. Note: The online search feature in EndNote 20 has been much improved.
Then click the + sign in a circle on the upper right above the references. The reference(s) will be added into your library.
If you find the desired reference(s), simply highlight the reference(s) you would like to keep. If too many items were retrieved, you may either refine your search by adding more search terms or click Clear search and rerun the search with a refined search strategy. In this search mode, I usually search by title in order to increase the likelihood to get a matching item. The Search interface on the right will reflect PubMed search boxes. Click on PubMed (NLM) under ONLINE SEARCG on the left navigation pane. Users need to choose the Online Search Mode to avoid putting irrelevant references in their libraries). (Note: in EndNote X9 and earlier, there are three icons: Local Library Mode, Online Search Mode (Temporary Library), and Integrated Library & Online Search Mode on the upper left corner. First, you need to have an internet connection. However, I would not recommend using this search function if you are performing a topic search, which should be conducted in a relevant database. 
This is particularly easy when the database is publicly accessible, for example: PubMed, so that you do not need to authenticate your access. If you are looking for a particular reference, you may search for it in a remote database directly from EndNote.
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